Sunday, December 2, 2012

A better way to make chemicals? Technique for observing 'mechanochemical' synthesis could boost green chemistry

ScienceDaily (Dec. 2, 2012) ? Bulk solvents, widely used in the chemical industry, pose a serious threat to human health and the environment. As a result, there is growing interest in avoiding their use by relying on "mechanochemistry" -- an energy-efficient alternative that uses high-frequency milling to drive reactions. Because milling involves the intense impact of steel balls in rapidly moving jars, however, the underlying chemistry is difficult to observe.

Now, for the first time, scientists have studied a milling reaction in real time, using highly penetrating X-rays to observe the surprisingly rapid transformations as the mill mixed, ground, and transformed simple ingredients into a complex product. This research, reported Dec. 2 in Nature Chemistry, promises to advance scientists' understanding of processes central to the pharmaceutical, metallurgical, cement and mineral industries -- and could open new opportunities in "green chemistry" and environmentally friendly chemical synthesis.

The international team of researchers was led by Tomislav Fri??i? of McGill University in collaboration with Ivan Halasz from the University of Zagreb in Croatia, and scientists from the University of Cambridge, the Max-Planck-Institute for Solid State Research in Stuttgart, Germany, and the European Synchrotron Radiation Facility (ESRF) in Grenoble, France.

While mechanical action can break chemical bonds -- for example, in the wear and tear of textile fibers -- mechanical force can also be used to synthesize new chemical compounds and materials. In recent years, ball milling has become increasingly popular in the production of highly complex chemical structures. In such synthesis, steel balls are shaken with the reactants and catalysts in a rapidly vibrating jar. Chemical transformations take place at the sites of ball collision, where impact causes instant "hot spots" of localized heat and pressure. This is difficult to model and, without access to real time reaction monitoring, mechanochemistry remained poorly understood.

"When we set out to study these reactions, the challenge was to observe the entire reaction without disturbing it, in particular the short-lived intermediates that appear and disappear under continuous impact in less than a minute," says Fri??i?, an assistant professor in McGill's Department of Chemistry.

The team of scientists chose to study mechanochemical production of the metal-organic framework ZIF-8 from the simplest and non-toxic components. Materials such as ZIF-8 are rapidly gaining popularity for their ability to capture large amounts of CO2; if manufactured cheaply and sustainably, they could become widely used for carbon capture and storage, catalysis and even hydrogen storage.

"The team came to the ESRF because of our high-energy X-rays capable of penetrating 3 mm thick walls of a rapidly moving reaction jar made of steel, aluminium or plastic. The X-ray beam must get inside the jar to probe the mechanochemical formation of ZIF-8, and then out again to detect the changes as they happened," says Simon Kimber, a scientist at the European Synchrotron Radiation Facility (ESRF) in Grenoble, who is a member of the team. This unprecedented methodology enabled the real-time observation of reaction kinetics, reaction intermediates and the development of their respective nanoparticles.

In principle, this technique could be used to study all types of chemical reactions in a ball mill, and optimize them for processing in a range of industries. "That would translate into good news for the environment, for industry -- and for consumers," Fri??i? says.

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The above story is reprinted from materials provided by McGill University, via EurekAlert!, a service of AAAS.

Note: Materials may be edited for content and length. For further information, please contact the source cited above.


Journal Reference:

  1. Tomislav Fri??i?, Ivan Halasz, Patrick J. Beldon, Ana M. Belenguer, Frank Adams, Simon A.J. Kimber, Veijo Honkim?ki, Robert E. Dinnebier. Real-time and in situ monitoring of mechanochemical milling reactions. Nature Chemistry, 2012; DOI: 10.1038/nchem.1505

Note: If no author is given, the source is cited instead.

Disclaimer: Views expressed in this article do not necessarily reflect those of ScienceDaily or its staff.

Source: http://feeds.sciencedaily.com/~r/sciencedaily/most_popular/~3/fBNQ2rCEehg/121202164432.htm

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Williamsburg, Classes, Activities, Recreational Sports, Art, Dance ...

Youth

REC Connect Winter Break Program(grades K-5)

Dec. 26, 27, 28 & 31; 7 a.m.-6 p.m.

Full-time (4 days) $90; $85 JC/W residents + field trip fees

Part-time (3 days or less) $70; $65 residents + field trip fees

Rawls Byrd Elementary School

Dependable and safe fun, games, fun fitness activities, creative crafts, interactive reading, team projects, music and daily field trips are just a few great program features!Info: jamescitycountyva.gov/recreation or call 757-259-4200.

Kid?s Holiday Dessert Camp (ages 7-12), New!

Thursday, Friday, & Saturday, Dec. 27-29 10 a.m.-noon

Thursday, Friday, & Saturday, Dec. 27-29 1:30-3:30 p.m.

$65/session; $60 for JC/W residents

James City County Recreation Center

Teens

Reaching for Success (grades 9-12)

Saturday, Dec. 1, 10 a.m. ? 2 p.m.

$25; $20 for JC/W residents

James City County Recreation Center

Winter Break Happenings (grades 6-12)

Rollin? Down the Lane

Wednesday, Dec. 26, 7 a.m. ? 6 p.m.

$35; $30 for JC/W residents

James City County Recreation Center

Now Showing?

Thursday, Dec. 27, 7 a.m. ? 6 p.m.

$35; $30 for JC/W residents

James City County Recreation Center

Cold as Ice

Friday, Dec. 28, 7 a.m. ? 6 p.m.

$35; $30 for JC/W residents

James City County Recreation Center

Tag ? You?re Out!

Monday, Dec. 31, 7 a.m. ? 6 p.m.

$35; $30 for JC/W residents

James City County Recreation Center

Inclusion

Teensational Socials: Holiday Shopping (ages 13-21 with disabilities)

Saturday, Dec. 15, 1-3:30 p.m.

$20; $15 for JC/W residents

James City County Recreation Center

Adults

Little Known Secrets of Paying for College (for parents)

Tuesday, Dec. 4, 6-8:30 p.m.

$30; $25 for JC/W residents (per set of parents)

James City County Recreation Center

Learn how to attend private schools for the same ?cost? as in-state schools, pay for college in the most efficient and effective manner, qualify for maximum financial aid package and gain an insider?s view of the college admissions process. Register by Nov. 29. Info:jamescitycountyva.gov/recreation or call 757-259-4200.

Color Mixing for Artists (ages 16+), New

Thursdays, Dec. 6 & 13, 10 a.m.-noon

$50; $45 for JC/W residents

James City County Recreation Center

Learn how to combine colors consistently and create a balanced palette. Learn about paint properties for all mediums and about choosing pigments. All materials provided. Info: jamescitycountyva.gov/recreation or call 757-259-4200.

Dance

Beginning Ballet

Thursdays, Dec. 6-Jan. 31, 2-3 p.m.

$25; 20 for JC/W residents

This class is intended for beginners, yet will be appropriate for anyone who wants to enjoy a relaxing exercise class. Ballet shoes are recommended, but not required. Info: jamescitycountyva.gov/recreation or call 757-259-4200.

Low Impact Tap

Mondays, Dec. 10-Jan. 28 (no class 12/24), 2-3 p.m.

$25; 20 for JC/W residents

James City County Recreation Center

We?ll combine both seated and standing tap dance exercises that allow anyone to enjoy dancing! Tap shoes are recommended, but not required. Info:jamescitycountyva.gov/recreation or call 757-259-4200.

Beginning Jazz

Wednesdays, Dec. 12-Jan.30, 7-8 p.m.

$25; 20 for JC/W residents

James City County Recreation Center

Jazz has its roots in African and Caribbean dance and lends itself to being great aerobic exercise as well as exercise for the mind. Jazz shoes are recommended, but not required. Info: jamescitycountyva.gov/recreation or call 757-259-4200.

Fitness

Evening Fitness Classes

Evening classes include Kickboxing, Zumba, Power Yoga, Cardio Tap dancing and Strength Training. Child care is available on Mondays and Wednesdays from 5-8 p.m. at the James City County Recreation Center. Call 757-259-4200 for details or visit us atjamescitycountyva.gov/recreation.

Source: http://williamsburgfamiliessports.blogspot.com/2012/11/jcc-parks-and-recreation-in-december.html

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Source: http://ibitylysin.wordpress.com/2012/12/01/williamsburg-classes-activities-recreational-sports-art-dance/

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Saturday, December 1, 2012

Japan Society: Japan News Roundup: Tsunami Debris Relief ...


? Japan will give the U.S. National Oceanic and Atmospheric Administration $5 million ?to help with collection and disposal of marine debris from its March 2011 tsunami disaster? (BusinessWeek). Timely news as debris is expected to land in Hawaii soon, specifically on a beach where an estimated 20 tons of current-carried garbage already washes ashore every year (NBC).

? Japan put many 3/11 reconstruction projects not linked to disaster zones on hold "after criticism the spending was not directly related to recovery from the disasters" (Associated Press). With $148 billion earmarked for ?unrelated projects, including subsidies for a contact lens factory in another region and research whaling,? the hold frees up only $210 million. In addition, the government plans to sell off some 56,000 homes lent cheaply to officials to raise approximately $2.1 billion for reconstruction (Bloomberg News).

? A United Nations envoy urged Japan to do more for residents and workers affected by the Fukushima nuclear crisis, citing over-emphasized optimism on radiation risks and lack of access to health check results as major ongoing problems. (Associated Press)

? With elections just weeks away, Japan's ruling party promised "cool-headed and practical" diplomacy in contrast with the opposition?s hawkish rhetoric, and restated its goal of phasing out nuclear power by the 2030s (Reuters). Japan unveiled a $11bn stimulus package, "its second round of stimulus in a little more than a month" (Financial Times). Meanwhile, Shiga Governor Yukiko Kada formed a new political group ?that aims to get Japan out of nuclear power, create more opportunities for women and promote a work-life balance that makes it easier for families to raise children? (Japan Times). Political powerhouse Ichiro Ozawa has joined.

? None of the candidates have won the hearts (or votes) of those in the tsunami-devastated region, who feel reconstruction has fallen off the political agenda (Reuters). "Many of the 159,000 people who fled their towns?are finally accepting that it may take decades, perhaps generations, before their town could be restored to anything like it was before the disaster? (New York Times).

? The Senkaku/Diaoyu island dispute between Japan and China ?has affected a broad cross-section of Japanese business, from cars to cosmetics. But perhaps the biggest blow has been to tourism?, with JNTO reporting Chinese tourism down in 33% from 2011. (Wall Street Journal)

? U.S. commanders are telling troops in Japan to ?put a cork in it? (TIME) and ?buddy up? (WSJ), after a number of arrests and embarrassing incidents. America?s highest-ranking military officer in Japan said ?the two countries are considering such countermeasures as joint U.S.-Japanese patrols and a ?hotline? in Okinawa for reporting troop misbehavior to U.S. military law enforcement officials? though ?he opposed reopening the status of forces agreement, an accord on the legal jurisdictions for American troops that has long been a lightning rod for anti-U.S. base activists.?

? In an annual government survey, Japan's feelings for the U.S., Russia and India are up, while views on China and South Korea "sank to their lowest levels in decades".

? People: Forbes highlights more of The Nikkei's top 100 people having the greatest influence on Japan?s future; the first Japanese-American woman senator vows to push Japan ties (Asiance Magazine); now in her 70s, Yoko Ono carves new niches in her life, from fighting world hunger to revolutionizing men's fashion (NYT); Forbes profiles Ernie Higa, the Wendy's Japan executive re-launching and revolutionizing the brand across the pacific (when talking about the country?s decline, he notes ?Japan is still alive. It?s the third-biggest economy, and you can still succeed here by finding the right niche and adapting?).

? Seascapes: Tokyo activists rallied against dolphin and whale hunts over the weekend, part of demonstrations to be held around the world (AFP), Japan on a quest to make bluefin tuna more sustainable (The Atlantic), meditation on ama, Japan's free diving 'sea women' (NYT).

South China Morning Post interviewed the authors of Strong in the Rain, the "harrowing but compassionate" collection of stories from tsunami victims. "There was a sense among many Tohoku people I met that telling their stories to journalists was grandstanding. They viewed their suffering as nothing special, compared to others," said one author.

? Language Lesson: Japan Times looks at "notable negatives" and other Japanese linguistic oddities, starting with the famous monkeys Mizaru, Kikazaru and Iwazaru (of "see/hear/speak no evil fame"). How did they get their names? "The negative verb inflexion -zaru, which happens to be a homonym for saru (monkey)."

? A look at the "sparkly names" trend in Japan favoring pop culture christenings for kids. (Kotaku)

? New book sheds light on 'grim' realities of mental healthcare in Japan. (Japan Times)

? Reuters weighs in on sumo's decline in 'age of convenience'.

? A 'floating' high-speed train unveiled in Tokyo is set to hit tracks in 2027 and cut travel time in more than half. (Discovery)

? Food: For the sixth consecutive year, Japan was awarded the most Michelin three-star rated restaurants in the world, ?though the number slipped to 14 from 16? (Reuters); with the adage sake "never fights with food", chefs outside of Japan are beginning to pair the libation with non-Japanese food (BBC); one of Japan's top airlines will offer KFC on fligths from Japan to U.S. and Europe over the winter holidays. (Business Insider); the Washington Post examined ji-biru, Japanese craft beer, one of "Japan?s least famous but most exciting gastronomic exports."

? The legacy of 007 in Japan: ?James Bond made his official Japan debut in ?You Only Live Twice?: The gentleman spy came to Tokyo and Fukuoka, saw some sumo, consorted with ninja and got intimate with two homegrown Bond girls? (Japan Times). In a plot fit for a Bond flick, Japan?s Aerospace Exploration Agency said that plans for a new solid-fuel rocket were stolen from computers (NYT).

? Tis the Season: ?On a recent weekend, 88 Santa wannabes packed the school in Tokyo's fashionable Roppongi district for a crash course in how to behave as ?Santa-san,? as the man in red is known in Japan.?

? Japanese toymaker plans to launch one-person electric helicopter next year. (WIRED)

? No plans for the weekend? Here's how to make Gudnam out of electrical plugs. (Rocketnews24)

? Two from Kotaku: The tiny might of 21st Century netsuke, and Japan's terrifying melon bear.

--SJ

Labels: news

Source: http://japansocietyny.blogspot.com/2012/11/japan-news-roundup-tsunami-debris.html

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Kenya village pairs AIDS orphans with grandparents

In this photo taken Wednesday, Nov. 21, 2012, a young schoolboy makes handstands during break in the yard of the Hot Courses Primary School, in the village of Nyumbani which caters to children who lost their parents to HIV, and grandparents who lost their children to HIV, with the bookend generations taking care of one another, in Kenya. Saturday, Dec. 1, is World AIDS Day, and UNAIDS says that as of 2011 an estimated 23.5 million people living with HIV resided in sub-Saharan Africa, representing 69 percent of the global HIV burden, with eastern and southern Africa the hardest-hit regions. (AP Photo/Ben Curtis)

In this photo taken Wednesday, Nov. 21, 2012, a young schoolboy makes handstands during break in the yard of the Hot Courses Primary School, in the village of Nyumbani which caters to children who lost their parents to HIV, and grandparents who lost their children to HIV, with the bookend generations taking care of one another, in Kenya. Saturday, Dec. 1, is World AIDS Day, and UNAIDS says that as of 2011 an estimated 23.5 million people living with HIV resided in sub-Saharan Africa, representing 69 percent of the global HIV burden, with eastern and southern Africa the hardest-hit regions. (AP Photo/Ben Curtis)

In this photo taken Wednesday, Nov. 21, 2012, children attend an outdoor Christian prayer session in front of a mural on the side of the meeting hall in the village of Nyumbani which caters to children who lost their parents to HIV, and grandparents who lost their children to HIV, with the bookend generations taking care of one another, in Kenya. Saturday, Dec. 1, is World AIDS Day, and UNAIDS says that as of 2011 an estimated 23.5 million people living with HIV resided in sub-Saharan Africa, representing 69 percent of the global HIV burden, with eastern and southern Africa the hardest-hit regions. (AP Photo/Ben Curtis)

In this photo taken Wednesday, Nov. 21, 2012, grandmother Janet Kitheka, 63, center, collects her adopted "grand-daughter" Lucy, 13, right, at the end of the school day in the yard of the Hot Courses Primary School, in the village of Nyumbani which caters to children who lost their parents to HIV, and grandparents who lost their children to HIV, with the bookend generations taking care of one another, in Kenya. Saturday, Dec. 1, is World AIDS Day, and UNAIDS says that as of 2011 an estimated 23.5 million people living with HIV resided in sub-Saharan Africa, representing 69 percent of the global HIV burden, with eastern and southern Africa the hardest-hit regions. (AP Photo/Ben Curtis)

In this photo taken Wednesday, Nov. 21, 2012, children attend morning assembly in the yard of the Hot Courses Primary School, in the village of Nyumbani which caters to children who lost their parents to HIV, and grandparents who lost their children to HIV, with the bookend generations taking care of one another, in Kenya. Saturday, Dec. 1, is World AIDS Day, and UNAIDS says that as of 2011 an estimated 23.5 million people living with HIV resided in sub-Saharan Africa, representing 69 percent of the global HIV burden, with eastern and southern Africa the hardest-hit regions. (AP Photo/Ben Curtis)

In this photo taken Wednesday, Nov. 21, 2012, children sing the lullaby "Twinkle, Twinkle, Little Star" during class at the Hot Courses Primary School, in the village of Nyumbani which caters to children who lost their parents to HIV, and grandparents who lost their children to HIV, with the bookend generations taking care of one another, in Kenya. Saturday, Dec. 1, is World AIDS Day, and UNAIDS says that as of 2011 an estimated 23.5 million people living with HIV resided in sub-Saharan Africa, representing 69 percent of the global HIV burden, with eastern and southern Africa the hardest-hit regions. (AP Photo/Ben Curtis)

(AP) ? There are no middle-aged people in Nyumbani. They all died years ago, before this village of hope in Kenya began. Only the young and old live here.

Nyumbani was born of the AIDS crisis. The 938 children here all saw their parents die. The 97 grandparents ? eight grandfathers among them ? saw their middle-aged children die. But put together, the bookend generations take care of one another.

Saturday is World AIDS Day, but the executive director of the aid group Nyumbani, which oversees the village of the same name, hates the name which is given to the day because for her the word AIDS is so freighted with doom and death. These days, it doesn't necessarily mean a death sentence. Millions live with the virus with the help of anti-retroviral drugs, or ARVs. And the village she runs is an example of that.

"AIDS is not a word that we should be using. At the beginning when we came up against HIV, it was a terminal disease and people were presenting at the last phase, which we call AIDS," said Sister Mary Owens. "There is no known limit to the lifespan now so that word AIDS should not be used. So I hate World AIDS Day, follow? Because we have moved beyond talking about AIDS, the terminal stage. None of our children are in the terminal stage."

In the village, each grandparent is charged with caring for about a dozen "grandchildren," one or two of whom will be biological family. That responsibility has been a life-changer for Janet Kitheka, who lost one daughter to AIDS in 2003. Another daughter died from cancer in 2004. A son died in a tree-cutting accident in 2006 and the 63-year-old lost two grandchildren in 2007, including one from AIDS.

"When I came here I was released from the grief because I am always busy instead of thinking about the dead," said Kitheka. "Now I am thinking about building a new house with 12 children. They are orphans. I said to myself, 'Think about the living ones now.' I'm very happy because of the children."

As she walks around Nyumbani, which is three hours' drive east of Nairobi, 73-year-old Sister Mary is greeted like a rock star by little girls in matching colorful school uniforms. Children run and play, and sleep in bunk beds inside mud-brick homes. High schoolers study carpentry or tailoring. But before 2006, this village did not exist, not until a Catholic charity petitioned the Kenyan government for land on which to house orphans.

Everyone here has been touched by HIV or AIDS. But only 80 children have HIV and thanks to anti-retroviral drugs, none of them has AIDS.

"They can dream their dreams and live a long life," Owens said.

Nyumbani relies heavily on U.S. funds but it is aiming to be self-sustaining.

The kids' bunk beds are made in the technical school's shop. A small aquaponics project is trying to grow edible fish. The mud bricks are made on site. Each grandparent has a plot of land for farming.

The biggest chunk of aid comes from the United States President's Emergency Plan for AIDS Relief (PEPFAR), which has given the village $2.5 million since 2006. A British couple gives $50,000 a year. A tree-growing project in the village begun by an American, John Noel, now stands six years from its first harvest. Some 120,000 trees have already been planted and thousands more were being planted last week.

"My wife and I got married as teenagers and started out being very poor. Lived in a trailer. And we found out what it was like to be in a situation where you can't support yourself," he said. "As an entrepreneur I looked to my enterprise skills to see what we could do to sustain the village forever, because we are in our 60s and we wanted to make sure that the thousand babies and children, all the little ones, were taken care of."

He hopes that after a decade the timber profits from the trees will make the village totally self-sustaining.

But while the future is looking brighter, the losses the orphans' suffered can resurface, particularly when class lessons are about family or medicine, said Winnie Joseph, the deputy headmaster at the village's elementary school. Kitheka says she tries to teach the kids how to love one another and how to cook and clean. But older kids sometimes will threaten to hit her after accusing her of favoring her biological grandchildren, she said.

For the most part, though, the children in Nyumbani appear to know how lucky they are, having landed in a village where they are cared for. An estimated 23.5 million people in sub-Saharan Africa have HIV as of 2011, representing 69 percent of the global HIV population, according to UNAIDS. Eastern and southern Africa are the hardest-hit regions. Millions of people ? many of them parents ? have died.

Kitheka noted that children just outside the village frequently go to bed hungry. And ARVs are harder to come by outside the village. The World Health Organization says about 61 percent of Kenyans with HIV are covered by ARVs across the country.

Paul Lgina, 14, contrasted the difference between life in Nyumbani, which in Swahili means simply "home," and his earlier life.

"In the village I get support. At my mother's home I did not have enough food, and I had to go to the river to fetch water," said Lina, who, like all the children in the village, has neither a mother or a father.

When Sister Mary first began caring for AIDS orphans in the early 1990s, she said her group was often told not to bother.

"At the beginning nobody knew what to do with them. In 1992 we were told these children are going to die anyway," she said. "But that wasn't our spirit. Today, kids we were told would die have graduated from high school."

___

On the Internet:

http://www.trees4children.org/

Associated Press

Source: http://hosted2.ap.org/APDEFAULT/b2f0ca3a594644ee9e50a8ec4ce2d6de/Article_2012-11-30-Kenya-AIDS%20Village/id-af520cb1f96147f3be37e62e22724796

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Infy shifts US listing to NYSE

Mumbai, Nov. 30: Infosys is preparing to bid goodbye to Nasdaq.

The Bangalore-based technology giant, which was the first Indian company to list on the tech-heavy Nasdaq in 1999, has decided to move its American depositary shares (ADS) to the New York Stock Exchange.

A statement from the company late in the evening said that Infosys ADS will begin trading on the NYSE Euronext markets in the US under the ticker symbol "INFY" on December 12.

The statement added that until the transfer was completed, Infosys ADS would continue to trade in the US under the ticker symbol INFY on the Nasdaq. Once the separate Euronext listing process is complete, Infosys ADS will begin trading on the NYSE Euronext markets in Paris and London.

The NYSE Euronext listing, however, will not change Infosys' float, share/ADR count and capital structure.

Infosys said the main objective behind the transfer was to widen its investor base.

"Our decision to transfer our ADS listing to the NYSE is motivated by a desire to leverage the NYSE Euronext partnership to empower our investor base, increase access to our stock for European investors and broaden the trading window available for our global investors," S. D. Shibulal, CEO and MD, Infosys said.

Other Indian companies listed on the Nasdaq include Cognizant and Rediff.

Source: http://news.yahoo.com/infy-shifts-us-listing-nyse-220116104--finance.html

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Let's Talk About How 'Looper' Should Have Ended

LOS ANGELES (Reuters) - Michael Jackson's father, Joe Jackson, has suffered a stroke but is OK and resting in a Las Vegas hospital, a family friend said on Thursday. "He was doing well and says he's feeling OK," close family friend Brian Oxman told Reuters. Oxman, Michael Jackson's one-time attorney, said the 83-year-old patriarch of the pop music family started experiencing weakness on Wednesday while walking in a park near his home and was later admitted to a hospital. Jackson has a history of strokes, Oxman said. "He was talking fine," Oxman added. "He sounded excellent to me." A former ...

Source: http://news.yahoo.com/lets-talk-looper-ended-221849985.html

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